Polymer Surface Dynamics

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Okano, in: Biomedical Polymers E. Goldberg and A. Nakajima, eds. Brier-Russell, E. Salzman, J. Lindon, R. Handin, E. Merrill, A. Dincer, and J. Wu, Interaction of blood with model surfaces J. Colloid Interface Sci. Thesis, University of Utah, August, Ledwith and A.

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North, eds. Armeniades and E. Kaufman, ed. Richardson and N.

Three Regimes of Polymer Surface Dynamics under Crowded Conditions - Dimensions

Savill, What information will DSC give on glassy polymers? Pethrick, Molecular motion in semi-flexible macromolecules, Sci. Cowie, Relaxation processes in the glassy state: molecular aspects, J. B18 , — Brandrup and E.

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Immergut, eds. Brostrom, D. Coleman, D. Gregonis, and J. Andrade, Thermal analysis of polymethacrylates, Makromol. Gillham, S. Standicki, and Y. Hazony, Low-frequency thermomechanical spectrometry of polymeric materials: tactic poly methyl methacrylates , J. McCrum, B. Read, and G. Woodward and F.


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Bovey, eds. Series Braun and J. Guillet, Study of polymers by inverse gas chromatography, Adv. Guillet, Studies of polystyrene in the region of the glass transition temperature by inverse gas chromatography, Macromolecules 8 , — Kessaissia, E. Papirer, and J. Donnet, Molecular transitions of alkyl chains grafted onto silicas observed by gas chromatography, J. Schreiber and M. Croucher, Surface characteristics of solvent-cast polymers, J.

Abstract Studies show that dynamical properties of ultra-thin polymer films deviate from those of bulk materials. Despite some controversial issues, there is growing evidence indicating that the interfacial properties play a key role for observed dynamical anomalies. However, how and how much the interfacial properties affect the average dynamics of the nanometer scale systems are still elusive.

In this work, we developed several novel techniques to investigate near-free-surface dynamics of thin polymer films. We used nano gold particle embedding to study PS surface dynamics: enhanced surface dynamics and weak temperature dependence were observed for the surface region; a depth profile with the nm resolution was observed; viscous liquid-like and soft solid-like properties were observed in the first 5.

We developed a novel nano rheology AFM technique to study the near-free-surface dynamics of thin polymer films: enhanced near-free-surface dynamics with weak temperature dependence are observed for PVAc films, which is similar with the PS case.

Gillham, S. Standicki, and Y.

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Hazony, Low-frequency thermomechanical spectrometry of polymeric materials: tactic poly methyl methacrylates , J. McCrum, B. Read, and G. Woodward and F. Bovey, eds. Series Braun and J. Guillet, Study of polymers by inverse gas chromatography, Adv. Guillet, Studies of polystyrene in the region of the glass transition temperature by inverse gas chromatography, Macromolecules 8 , — Kessaissia, E.

Papirer, and J. Donnet, Molecular transitions of alkyl chains grafted onto silicas observed by gas chromatography, J. Schreiber and M. Croucher, Surface characteristics of solvent-cast polymers, J.

Classes in Polymer Dynamics - 22 Viscosity

Lipatov and L. Howard and R. Shanks, Influence of filler particles on the mobility of polymer molecules, J.

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Surface dynamics in rubbed polymer thin films probed with optical birefringence measurements

Sci, Chem. A17 , — Yim, R. Chahal, and L. Pierre, Effect of polymer-filler interaction energy on the Tg of filled polymers, J. Peyser and W. Bascom, Effect of filler and cooling rate on the glass transition of polymers, J. B13 , — Pennings and B.

Bosman, Relaxation of the surface energy of solid polymers, Colloid Polym. Carre and H. Yasuda, A. Sharma, and T. Yasuda, Effect of orientation and mobility of polymer molecules at surfaces on contact angle and its hysteresis, J. Physics 19 , — Ke, ed.

Fox, P. Taylor, W. Zisman, Polyorganosiloxanes: surface active properties, Ind. Owen, The surface activity of silicones, Ind. Okawa, B. Ohara, Relationship between frictional electrification and molecular motion of polymers, J. Electrostatics 9 , — Klein and P.

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